阅读说明：本技术 一种青草药护肤品的配方及其制备方法 (Formula and preparation method of green herbal skin care product ) 是由 李艳 李梓源 章文浩 孙学华 范冠宝 于 2021-07-31 设计创作，主要内容包括：本发明提出了一种青草药护肤品,按重量百分比计算,具体配方为：忧遁草纯露1-5％,鹧鸪茶纯露0.5-3％,九里香纯露0.5-3％,烟酰胺0.5-1％,三甲基甘氨酸0.3-2％,海藻酸钠0.05-0.2％,透明质酸0.01-0.05％,余量为矿泉水。本发明制备获得的青草药护肤品具有保湿补水,控油祛痘,改善皮肤过敏的效果。(The invention provides a green herbal medicine skin care product, which comprises the following specific formula in percentage by weight: 1-5% of clinacanthus nutans hydrosol, 0.5-3% of francolin pintadeana tea hydrosol, 0.5-3% of murraya jasminorage hydrosol, 0.5-1% of nicotinamide, 0.3-2% of trimethylglycine, 0.05-0.2% of sodium alginate, 0.01-0.05% of hyaluronic acid and the balance of mineral water. The green herbal medicine skin care product prepared by the invention has the effects of moisturizing, controlling oil and removing acne and improving skin allergy.)

1. The green herbal skin care product is characterized by comprising the following specific formula in percentage by weight: 1-5% of clinacanthus nutans hydrosol, 0.5-3% of francolin pintadeana tea hydrosol, 0.5-3% of murraya jasminorage hydrosol, 0.5-2% of trimethylglycine, 0.5-1% of nicotinamide, 0.05-0.2% of sodium alginate, 0.01-0.05% of hyaluronic acid and the balance of mineral water.

2. The herbal skin care product according to claim 1, wherein the specific formula comprises, in weight percent: clinacanthus nutans hydrosol 4%, Mallotus furetianus hydrosol 2%, Murraya paniculata hydrosol 2%, trimethylglycine 1.5%, nicotinamide 1%, sodium alginate 0.08%, hyaluronic acid 0.03%, and mineral water in balance.

3. The green herbal skin care product of claim 1, wherein the clinacanthus nutans hydrolat is extracted from stems and leaves of clinacanthus nutans and fresh flowers at a weight ratio of 10: 1-3.

4. The herbal skin care product of claim 1, wherein the molecular weight of the hyaluronic acid is small molecular weight, specifically 300000-500000.

5. The green herbal skin care product of claim 1, wherein the clinacanthus nutans hydrolat is extracted by the following method:

step 1: selecting fresh Clinacanthus nutans stems and leaves of 4-6 months per year, Clinacanthus nutans fresh flowers, removing old leaves, cleaning, draining, putting into a distillation still, adding mineral water 2-3 times of the weight of Clinacanthus nutans, and adding sodium chloride 1-3% of the weight of Clinacanthus nutans;

step 2: heating and pressurizing for distillation, adding condensed water into the distillation kettle after the temperature in the kettle rises to a certain temperature, stopping heating, and collecting supernatant in the fraction, namely the clinacanthus nutans pure distillate.

6. The method for extracting clinacanthus nutans trub juice as claimed in claim 1 or 5, wherein in the step 2, the steam pressure is 0.02-0.08MPa, and the temperature in the kettle is stopped after reaching 55 ℃.

7. The herbal skin care product of claim 1, wherein the partridge tea hydrolat is extracted from the group consisting of:

step 1: selecting fresh Mallotus furetianus leaves, removing impurities, cleaning, draining, putting into a distillation still, and adding mineral water 2-3 times of the weight of Mallotus furetianus;

step 2: heating and pressurizing for distillation, adding condensed water into the distillation kettle after the temperature in the kettle rises to a certain temperature, stopping heating, and collecting supernatant in the fraction to obtain the Mallotus oblongifolius pure distillate.

8. The method for extracting Mallotus oblongifolius dunal tea as claimed in claim 1, wherein the steam pressure in step 2 is 0.1-0.2MPa, and the extraction is stopped when the temperature in the kettle reaches 70 ℃.

9. The herbal skin care product of claim 1, wherein the murraya jasminorage hydrolat is obtained by extracting the following:

step 1: selecting fresh Murraya koenigii, cleaning, draining, putting into a distillation still, adding mineral water 2-3 times of the weight of the Murraya koenigii, and adding absolute ethyl alcohol 5-10% of the weight of the Murraya koenigii;

step 2: heating and pressurizing for distillation, adding condensed water into the distillation kettle after the temperature in the kettle rises to a certain temperature, stopping heating, and collecting supernatant in the fraction to obtain the murraya paniculata hydrosol.

10. The method for extracting murraya jasminorage hydrosol as claimed in claim 1 or 9, wherein in the step 2, the steam pressure is 0.05-0.1MPa, and the extraction is stopped when the temperature in the kettle reaches 60 ℃.

Technical Field

The invention relates to the field of daily chemicals, in particular to a formula of a green herbal skin care product and a preparation method thereof.

Background

Li Wang Cao, also known as Clinacanthus nutans, is a wild shrub-like herbaceous plant growing in low-altitude sparse forests near the equator or in moist sandy soil in shrubs, and is extremely high in amino acids and chlorophyll. And displaying according to the test result: clinacanthus nutans is nontoxic and contains lupeol, betulin, pentacyclic triterpene compound, Beta sitosterol, calcium element, and flavonoid with high content. The Li nationality is mainly produced in tropical rain forest areas in Hainan China, Li nationality is the resident of the original position of the Hainan island, Li nationality medicine also has a long history, Li Wang Cao is the medicine for Li Wang who tributes to Li Wang at the earliest time and is called as one of Li Jia Sanbao.

Clinacanthus nutans is sweet, pungent, slightly bitter and neutral in flavor and enters liver and kidney meridians. Is a wild shrub-like herbaceous plant growing in low-altitude sparse forests near the equator or in moist sandy soil within a bush, and is extremely high in amino acids and chlorophyll. Has effects of clearing away heat and toxic materials, removing blood stasis, relieving swelling, relieving inflammation, relieving hangover, preventing cancer, improving blood flow state of the whole body, enhancing myocardial contractility, and improving blood pressure, and is rich in protein and high in nutritive value. The traditional Chinese medicine composition is used for treating nephritis, renal atrophy, renal failure and renal calculus, is a salvage for patients with kidney diseases, and also can be used for treating swelling and pain of throat, hepatitis, jaundice, skin diseases, hypertension, hyperglycemia, hyperlipidemia, gastritis and rheumatic arthralgia, and has a good treatment effect on various cancers. Li Wang Cao, also known as Clinacanthus nutans, academic name: crocodile flower.

The Mallotus furetianus tea has the functions of clearing away heat and toxic materials, clearing away heat, quenching thirst, promoting digestion and benefiting gallbladder.

The murraya paniculata, also known as cayenne pepper, murraya paniculata and the like, is evergreen shrub of murraya of Rutaceae, can grow into a small arbor shape sometimes, has beautiful plant posture, beautiful branches and leaves and strong flower fragrance, contains chemical components similar to those of the murraya paniculata in roots, stems and leaves, contains essential oil in flowers, leaves and fruits of the murraya paniculata, has an oil yield of 0.25 percent, and can be used for cosmetic essence and food essence; the leaves can be used as flavoring; the branches and leaves are used as medicine, and have the effects of promoting qi circulation, relieving pain, promoting blood circulation, and removing blood stasis, and can be used for treating stomachache and rheumatalgia, and for external use, can be used for treating toothache, traumatic injury, insect bite, snake bite, etc.

Acne, comedo and pimple are collectively called as acne in medicine, and are common sebaceous gland chronic diseases, pimple mostly occurs in adolescence (about 16-30 years old), most of pimples are self-healed after adolescence, the morbidity of males is higher than that of females, and summer is more than that of winter. The hair-growing part is skin rich in sebaceous glands on the face, the upper chest and the back.

Conventional acne-removing products usually contain hormone drugs or acidic drugs, and have high skin irritation, which can damage the stratum corneum of the skin and finally cause the skin to be easily allergic due to the loss of the protection of the natural sebum membrane.

CN110063925A provides an acne-removing composition and a preparation method thereof, the acne-removing composition comprises, by weight, 5-100 parts of ethanol, 5-100 parts of glycerol, 0.05-70 parts of naringenin, 0.05-50 parts of chlorogenic acid, 0.05-50 parts of eucalyptus essential oil, 0.05-50 parts of eugenol, 0.05-50 parts of emodin, 0.05-50 parts of menthyl lactate, 0.05-50 parts of tea polyphenol, 0.05-50 parts of quercetin, 0.05-50 parts of periplaneta americana extract, 0.05-50 parts of allantoin and 0.05-50 parts of vitamin A acetate. The patent contains vitamin a, may damage the stratum corneum of the skin, and contains animal extracts, may easily cause allergy problems.

CN106852763A relates to a method for preparing acne-removing emulsion, which is prepared by mixing snail protein powder, fructus forsythiae extract, lithospermum extract, purslane extract, arbutin, magnolin extract, chamomile extract, aloe extract, platycladus orientalis extract, dandelion extract, turmeric extract, liquorice extract, oat beta glucan aqueous solution, gynostemma pentaphylla extract, lavender extract, gentian extract, sanguisorba extract, clove extract, pomegranate extract, vitamin C, raspberry glycoside, vitamin A, nicotinamide, high-content aloside (glycoside), rheum officinale extract, isooctyl palmitate, isopropyl palmitate, emulsifying wax, perfume and ionized water. The patent ingredient is complex, may cause skin allergy, and has poor moisturizing effect.

Disclosure of Invention

Therefore, the invention aims to provide a green herbal skin care product with the functions of moisturizing, controlling oil, removing acne and improving skin allergy and a preparation method thereof.

A green herbal medicine skin care product comprises the following specific formula in percentage by weight: 1-5% of clinacanthus nutans hydrosol, 0.5-3% of francolin pintadeana tea hydrosol, 0.5-3% of murraya jasminorage hydrosol, 0.5-2% of trimethylglycine, 0.5-1% of nicotinamide, 0.05-0.2% of sodium alginate, 0.01-0.05% of hyaluronic acid and the balance of mineral water.

Further, the clinacanthus nutans pure dew is extracted from clinacanthus nutans stems and leaves and fresh flowers, and the weight ratio of the stems to the leaves to the fresh flowers is 10: 1-3.

Further, the molecular weight of the hyaluronic acid is small molecular weight, specifically 300000-500000.

Further, the clinacanthus nutans hydrolat is obtained by extracting through the following method:

step 1: selecting fresh Clinacanthus nutans stems and leaves of 4-6 months per year, Clinacanthus nutans fresh flowers, removing old leaves, cleaning, draining, putting into a distillation still, adding mineral water 2-3 times of the weight of Clinacanthus nutans, and adding sodium chloride 1-3% of the weight of Clinacanthus nutans;

step 2: heating and pressurizing for distillation, adding condensed water into the distillation kettle after the temperature in the kettle rises to a certain temperature, stopping heating, and collecting supernatant in the fraction, namely the clinacanthus nutans pure distillate.

Further, in the step 2, the steam pressure is 0.02-0.08MPa, and the temperature in the kettle is stopped after reaching 55 ℃.

Further, the mallotus oblongifolius pure dew is obtained by extracting through the following method:

step 1: selecting fresh Mallotus furetianus leaves, removing impurities, cleaning, draining, putting into a distillation still, and adding mineral water 2-3 times of the weight of Mallotus furetianus;

step 2: heating and pressurizing for distillation, adding condensed water into the distillation kettle after the temperature in the kettle rises to a certain temperature, stopping heating, and collecting supernatant in the fraction to obtain the Mallotus oblongifolius pure distillate.

Further, in the step 2, the steam pressure is 0.1-0.2MPa, and the process is stopped when the temperature in the kettle reaches 70 ℃.

Further, the murraya jasminorage hydrosol is obtained by extracting through the following method:

step 1: selecting fresh Murraya koenigii, cleaning, draining, putting into a distillation still, adding mineral water 2-3 times of the weight of the Murraya koenigii, and adding absolute ethyl alcohol 5-10% of the weight of the Murraya koenigii;

step 2: heating and pressurizing for distillation, adding condensed water into the distillation kettle after the temperature in the kettle rises to a certain temperature, stopping heating, and collecting supernatant in the fraction to obtain the murraya paniculata hydrosol.

Further, in the step 2, the steam pressure is 0.05-0.1MPa, and the temperature in the kettle is stopped after reaching 60 ℃.

Compared with the prior art, the invention has the beneficial effects that:

1) the green herbal medicine skin care product prepared by the invention has the effects of moisturizing, controlling oil, removing acne and improving skin allergy;

2) the green herbal medicine skin care product is simple in preparation method and can be produced in batches.

Detailed Description

For clear and complete description of the technical solutions in the present invention, it is obvious that the inventor combines the embodiments to describe, but the following embodiments describe only some embodiments of the present invention, not all embodiments. All other embodiments, which can be derived by a person skilled in the art from the embodiments given herein without making any creative effort, shall fall within the protection scope of the present invention.

Example 1, formulation test:

the clinacanthus nutans pure distillate, the mallotus oblongifolius pure distillate and the murraya jasminorage pure distillate are prepared according to the following steps.

Clinacanthus nutans hydrolat:

step 1: selecting fresh Clinacanthus nutans stems and leaves of 4-6 months per year, Clinacanthus nutans fresh flowers, removing old leaves, cleaning, draining, putting into a distillation still, adding mineral water 2-3 times of the weight of Clinacanthus nutans, and adding sodium chloride 1-3% of the weight of Clinacanthus nutans;

step 2: heating and pressurizing for distillation under the steam pressure of 0.02-0.08MPa, adding condensed water into the distillation kettle when the temperature in the kettle reaches 55 ℃, stopping heating, and collecting supernatant in the distillate, namely the clinacanthus nutans pure distillate.

Partridge tea hydrolat:

step 1: selecting fresh Mallotus furetianus leaves, removing impurities, cleaning, draining, putting into a distillation still, and adding mineral water 2-3 times of the weight of Mallotus furetianus;

step 2: heating and pressurizing for distillation under the steam pressure of 0.1-0.2MPa until the temperature in the distillation kettle reaches 70 ℃, adding condensed water into the distillation kettle, stopping heating, and collecting supernatant in the fraction to obtain the Mallotus oblongifolius water.

Murraya paniculata hydrolat:

step 1: selecting fresh Murraya koenigii, cleaning, draining, putting into a distillation still, adding mineral water 2-3 times of the weight of the Murraya koenigii, and adding absolute ethyl alcohol 5-10% of the weight of the Murraya koenigii;

step 2: heating and pressurizing for distillation under the steam pressure of 0.05-0.1MPa, adding condensed water into the distillation kettle when the temperature in the kettle reaches 60 ℃, stopping heating, and collecting supernatant in the distillate to obtain the murraya paniculata hydrosol.

The preparation method of the hydrosol comprises the following steps:

weighing the clinacanthus nutans hydrolat, the mallotus furetianus hydrolat, the murraya jasminorage hydrolat, the trimethylglycine and the nicotinamide according to the following weight, adding mineral water, uniformly mixing, adding the sodium alginate and the hyaluronic acid, and stirring and mixing.

Sample 1:

clinacanthus nutans hydrosol 1%, Mallotus furetianus hydrosol 3%, Murraya paniculata hydrosol 1%, trimethylglycine 0.5%, nicotinamide 1%, sodium alginate 0.05%, hyaluronic acid 0.02%, and mineral water 93.43%.

Sample 2:

clinacanthus nutans hydrosol 2%, Caloglossa chinensis tea hydrosol 2%, Murraya koenigii hydrosol 0.5%, trimethylglycine 1%, nicotinamide 0.8%, sodium alginate 0.2%, hyaluronic acid 0.05%, and mineral water 93.45%.

Sample 3:

clinacanthus nutans hydrosol 3%, Mallotus furetianus hydrosol 1%, Murraya paniculata hydrosol 3%, trimethylglycine 2%, nicotinamide 0.5%, sodium alginate 0.15%, hyaluronic acid 0.04%, and mineral water 90.31%.

Sample 4:

clinacanthus nutans hydrosol 4%, Mallotus furetianus hydrosol 2%, Murraya paniculata hydrosol 2%, trimethylglycine 1.5%, nicotinamide 1%, sodium alginate 0.08%, hyaluronic acid 0.03%, and mineral water 89.39%.

Sample 5:

5% of clinacanthus nutans hydrosol, 0.5% of francolin pintada tea hydrosol, 2% of murraya paniculata hydrosol, 1.5% of trimethylglycine, 0.7% of nicotinamide, 0.1% of sodium alginate, 0.01% of hyaluronic acid and 90.19% of mineral water.

Sample 6:

7% of clinacanthus nutans hydrosol, 4% of mallotus nutans tea hydrosol, 4% of murraya jasminorage hydrosol, 2% of trimethylglycine, 1% of nicotinamide, 0.2% of sodium alginate, 0.05% of hyaluronic acid and 81.75% of mineral water.

Sample 7:

clinacanthus nutans hydrosol 3%, Mallotus furetianus hydrosol 6%, Murraya paniculata hydrosol 0.1%, trimethylglycine 0.2%, nicotinamide 0.2%, sodium alginate 0.2%, hyaluronic acid 0.02%, and mineral water 90.28%.

Sample 8:

clinacanthus nutans hydrosol 3%, Mallotus oblongifolius tea hydrosol 2%, sodium alginate 0.1%, hyaluronic acid 0.03%, and mineral water 94.87%.

Sample 9:

clinacanthus nutans hydrosol 3%, Mallotus oblongifolius tea hydrosol 2%, Murraya paniculata hydrosol 2% and mineral water 93%.

Sample 10:

2 percent of Mallotus furetianus pure distillate, 2 percent of Murraya paniculata pure distillate, 1.5 percent of trimethyl glycine, 1 percent of nicotinamide, 0.08 percent of sodium alginate, 0.03 percent of hyaluronic acid and 93.39 percent of mineral water.

Sample 11:

clinacanthus nutans hydrolat 4%, trimethylglycine 1.5%, nicotinamide 1%, sodium alginate 0.08%, hyaluronic acid 0.03%, and mineral water 93.39%.

Sample 12:

1.5 percent of trimethylglycine, 1 percent of nicotinamide, 0.08 percent of sodium alginate, 0.03 percent of hyaluronic acid and 97.39 percent of mineral water.

Sample No. 13:

100% of mineral water.

Example 2: the preparation process was varied according to the proportions given for sample 4.

Sample 14: when Clinacanthus nutans, Mallotus furetianus and murraya jasminorage syrup are prepared, the steam pressure is 0.05-0.1MPa, the heating is stopped until the temperature in the kettle reaches 100 ℃, and the rest processes are consistent with those of the sample 4.

Sample 15: when preparing the clinacanthus nutans, sodium chloride is not added; when the murraya jasminorage hydrolat is prepared, no ethanol is added; the rest of the procedure was identical to sample 4.

Samples 1-15 were tested.

Water replenishing and moisture preserving:

45 subjects were selected and divided into 15 groups of 3 persons each. After washing hands for 15min, smearing a hydrolat sample 1-15 on the inner side of the left arm of the subject, testing the moisture content of the skin, selecting the same position of the right arm as a blank control, and calculating the moisturizing effect by adopting the following formula. The average of 3 persons was calculated.

Moisturizing effect ═ 100% (left arm test value-right arm blank value)/right arm blank value%

The results are shown in Table 1.

Table 1:

the acne removing effect is as follows:

and evaluating the acne removing effect of the sample according to the evaluation method of the sample on the bacteriostatic effect of the propionibacterium acnes.

Culturing Propionibacterium acnes at 37 + -1 deg.C for 72 hr, eluting after bacterial colony grows to obtain 1 × 10⁸CFU/mL bacterial suspension, 0.2mL bacterial suspension added agarEvenly coating after flattening, and naturally drying. Soaking a circular filter paper sheet with the diameter of 5mm in the hydrolat of a test sample 1-15, taking out the filter paper after 5min, removing redundant samples, placing the soaked sample filter paper sheet on the surface of a flat plate, placing the flat plate upside down in an anaerobic tank, and culturing for 48h at 37 +/-1 ℃. The plate was removed and the size of the zone of inhibition was measured for each sample 1-15. The specific test results are shown in table 2:

table 2 (bacteriostatic diameter in mm):

	bacteriostatic diameter mm		Bacteriostatic diameter mm		Bacteriostatic diameter mm		Bacteriostatic diameter mm
								Blank space	0	Sample No. 4	21	Sample 8	12	Sample 12	1
Sample 1	17	Sample No. 5	19	Sample 9	8	Sample 13	0
								Sample 2	20	Sample No. 6	17	Sample 10	6	Sample 14	18
Sample 3	19	Sample 7	14	Sample 11	10	Sample 15	16

In conclusion, according to the method disclosed by the application, the green herbal medicine skin care product with the functions of moisturizing, controlling oil, removing acnes and improving skin allergy can be obtained.

The above description is only for the purpose of illustrating the preferred embodiments of the present invention and is not to be construed as limiting the invention, and any modifications, equivalents, improvements and the like that fall within the spirit and principle of the present invention are intended to be included therein.